Slice imaging of the photodissociation of acetaldehyde at 248 nm. Evidence of a roaming mechanism

Phys Chem Chem Phys. 2007 Dec 14;9(46):6123-7. doi: 10.1039/b708310f. Epub 2007 Oct 11.

Abstract

The photodissociation of acetaldehyde in the molecular channel yielding CO and CH(4) at 248 nm has been studied, probing different rotational states of the CO(nu = 0) fragment by slice ion imaging using a 2+1 REMPI scheme at around 230 nm. From the slice images, clear evidence of the co-existence of two different mechanisms has been obtained. One of the mechanisms is consistent with the well-studied conventional transition state in which CO products appear rotationally excited, and the second is consistent with a roaming mechanism. This roaming mechanism is characterized by a low rotational energy disposal into the CO fragment as well as by a very low kinetic energy release, corresponding to a high internal energy in the CH(4) counter-fragment.

Publication types

  • Research Support, Non-U.S. Gov't