Determination of ecabet in human plasma by high-performance liquid chromatography-tandem mass spectrometry

J Chromatogr B Analyt Technol Biomed Life Sci. 2008 Mar 1;863(2):223-8. doi: 10.1016/j.jchromb.2008.01.013. Epub 2008 Jan 16.

Abstract

This paper describes a simple, robust and cost-effective assay for the determination of ecabet in human plasma. After a simple step of protein precipitation using methanol, plasma samples were analyzed by reverse phase high-performance liquid chromatography-electrospray ionization-tandem mass spectrometry (HPLC-ESI-MS/MS) with valsartan as the internal standard (I.S.). Ecabet and the I.S. valsartan were separated on a Venusil MP C18 analytical column using methanol-10mM ammonium acetate (75:25, v/v, pH 3.0) as mobile phase at a flow rate of 1.0 mL/min. Ecabet and I.S. were eluted at 0.91 and 0.92 min, respectively, ionized in negative mode, and then detected by multiple reaction monitoring (MRM) essay. The MRM transitions of m/z 379.1-->m/z 277.1 and m/z 434.3-->m/z 350.1 were used to quantify ecabet and I.S., respectively. The assay was linear over the concentration range of 10-6000 ng/mL and was successfully applied to a pharmacokinetic study in healthy volunteers.

Publication types

  • Evaluation Study
  • Validation Study

MeSH terms

  • Abietanes / blood*
  • Abietanes / chemistry
  • Area Under Curve
  • Chromatography, High Pressure Liquid / instrumentation
  • Chromatography, High Pressure Liquid / methods*
  • Humans
  • Hydrophobic and Hydrophilic Interactions
  • Methanol / chemistry
  • Reference Standards
  • Reproducibility of Results
  • Sensitivity and Specificity
  • Spectrometry, Mass, Electrospray Ionization / methods
  • Tandem Mass Spectrometry / methods*
  • Tetrazoles / blood
  • Tetrazoles / chemistry
  • Valine / analogs & derivatives
  • Valine / blood
  • Valine / chemistry
  • Valsartan

Substances

  • Abietanes
  • Tetrazoles
  • ecabet
  • Valsartan
  • Valine
  • Methanol