Simultaneous analysis of FDG, ClDG and Kryptofix 2.2.2 in [18F]FDG preparation by high-performance liquid chromatography with UV detection

Nucl Med Biol. 2008 Feb;35(2):239-44. doi: 10.1016/j.nucmedbio.2007.11.003.

Abstract

A practical, sensitive and rapid analytical method was established and validated for chemical impurity tests of 2-deoxy-2-fluoro-d-glucose (FDG), 2-deoxy-2-chloro-d-glucose (ClDG) and Kryptofix 2.2.2 (K-222) in [18F]FDG. This method was based on precolumn derivatization with ultraviolet (UV) detection. FDG and ClDG were rapidly derivatized with 1-phenyl-3-methyl-5-pyrazolone in the presence of borate buffer at 40 degrees C, and the labeled derivatives and K-222 were separated by reversed-phase high-performance liquid chromatography and monitored by UV absorbance at 210 nm. After optimization of the conditions, FDG, ClDG and K-222 could be determined within 15 min and showed good performance in terms of sensitivity, linearity and reproducibility. This method could be successfully applied to the quality control test of [18F]FDG produced by a commercially available apparatus.

MeSH terms

  • Bridged Bicyclo Compounds, Heterocyclic / analysis*
  • Chromatography, High Pressure Liquid / methods*
  • Deoxyglucose / analogs & derivatives*
  • Deoxyglucose / analysis
  • Deoxyglucose / radiation effects
  • Drug Stability
  • Fluorodeoxyglucose F18 / analysis*
  • Fluorodeoxyglucose F18 / radiation effects
  • Pharmaceutical Preparations / analysis*
  • Pharmaceutical Preparations / radiation effects
  • Quality Control
  • Radiopharmaceuticals / analysis
  • Radiopharmaceuticals / radiation effects
  • Spectrophotometry, Ultraviolet / methods
  • Stereoisomerism

Substances

  • Bridged Bicyclo Compounds, Heterocyclic
  • Pharmaceutical Preparations
  • Radiopharmaceuticals
  • Fluorodeoxyglucose F18
  • 2-chloro-2-deoxyglucose
  • cryptating agent 222
  • Deoxyglucose