Treatment with DF 2162, a non-competitive allosteric inhibitor of CXCR1/2, diminishes neutrophil influx and inflammatory hypernociception in mice

Br J Pharmacol. 2008 May;154(2):460-70. doi: 10.1038/bjp.2008.94. Epub 2008 Mar 24.

Abstract

Background and purpose: Neutrophil migration into tissues is involved in the genesis of inflammatory pain. Here, we addressed the hypothesis that the effect of CXC chemokines on CXCR1/2 is important to induce neutrophil migration and inflammatory hypernociception.

Experimental approach: Mice were treated with a non-competitive allosteric inhibitor of CXCR1/2, DF 2162, and neutrophil influx and inflammatory hypernociception were assessed by myeloperoxidase assay and electronic pressure meter test, respectively, in various models of inflammation.

Key results: DF 2162 inhibited neutrophil chemotaxis induced by CXCR1/2 ligands but had no effect on CXCL8 binding to neutrophils. A single mutation of the allosteric site at CXCR1 abrogated the inhibitory effect of DF 2162 on CXCL-8-induced chemotaxis. Treatment with DF 2162 prevented influx of neutrophils and inflammatory hypernociception induced by CXCL1 in a dose-dependent manner. The compound inhibited neutrophil influx and inflammatory hypernociception induced by carrageenan, lipopolysaccharide and zymosan, but not hypernociception induced by dopamine and PGE(2). DF 2162 had a synergistic effect with indomethacin or the absence of TNFR1 to abrogate carrageenan-induced hypernociception. Treatment with DF 2162 diminished neutrophil influx, oedema formation, disease score and hypernociception in collagen-induced arthritis.

Conclusions and implications: CXCR1/2 mediates neutrophil migration and is involved in the cascade of events leading to inflammatory hypernociception. In addition to modifying fundamental pathological processes, non-competitive allosteric inhibitors of CXCR1/2 may have the additional benefit of providing partial relief for pain and, hence, may be a valid therapeutic target for further studies aimed at the development of new drugs for the treatment of rheumatoid arthritis.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Analgesics / pharmacology*
  • Analgesics / therapeutic use
  • Animals
  • Arthritis, Experimental / complications
  • Arthritis, Experimental / drug therapy
  • Benzeneacetamides / pharmacology*
  • Benzeneacetamides / therapeutic use
  • Cells, Cultured
  • Chemokine CXCL1 / metabolism
  • Chemotaxis, Leukocyte / drug effects
  • Cyclooxygenase Inhibitors / pharmacology
  • Dose-Response Relationship, Drug
  • Humans
  • Hyperalgesia / etiology
  • Hyperalgesia / immunology
  • Hyperalgesia / prevention & control*
  • Indomethacin / pharmacology
  • Inflammation / complications*
  • Inflammation / drug therapy
  • Inflammation / immunology
  • Interleukin-8 / metabolism
  • Male
  • Mesylates / pharmacology*
  • Mesylates / therapeutic use
  • Mice
  • Mice, Inbred C57BL
  • Mice, Inbred DBA
  • Mice, Knockout
  • Neutrophil Infiltration / drug effects*
  • Neutrophils / drug effects*
  • Neutrophils / immunology
  • Pain Measurement
  • Receptors, Interleukin-8A / antagonists & inhibitors*
  • Receptors, Interleukin-8A / genetics
  • Receptors, Interleukin-8A / metabolism
  • Receptors, Interleukin-8B / antagonists & inhibitors*
  • Receptors, Interleukin-8B / metabolism
  • Receptors, Tumor Necrosis Factor, Type I / genetics
  • Receptors, Tumor Necrosis Factor, Type I / metabolism
  • Transfection

Substances

  • 4-(2-amino-1-methyl-2-oxoethyl)phenyl trifluoromethanesulfonate
  • Analgesics
  • Benzeneacetamides
  • Chemokine CXCL1
  • Cyclooxygenase Inhibitors
  • Interleukin-8
  • Mesylates
  • Receptors, Interleukin-8A
  • Receptors, Interleukin-8B
  • Receptors, Tumor Necrosis Factor, Type I
  • Tnfrsf1a protein, mouse
  • Indomethacin