De novo synthesis of a D-galacturonic acid thioglycoside as key to the total synthesis of a glycosphingolipid from Sphingomonas yanoikuyae

Org Lett. 2008 Apr 17;10(8):1573-6. doi: 10.1021/ol800227b. Epub 2008 Mar 26.

Abstract

A concise synthesis of a differentially protected D-galacturonic acid (D-GalA) thioglycoside and the construction of a potent immunomodulating glycosphingolipid are described. The key steps of the synthesis are an Evans aldol reaction between a C4 aldehyde and a PMB-protected glycolyloxazolidinone as well as a tandem-PMB-deprotection/cyclization to thioglycosides. The key glycosylation step is optimized by varying the anomeric leaving group, the activating agent, and the solvent system.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Glycosphingolipids / chemical synthesis*
  • Sphingomonas / chemistry*
  • Thioglycosides / chemical synthesis*

Substances

  • Glycosphingolipids
  • Thioglycosides