Enzymatic characterization of 5-methylthioribulose-1-phosphate dehydratase of the methionine salvage pathway in Bacillus subtilis

Biosci Biotechnol Biochem. 2008 Apr;72(4):959-67. doi: 10.1271/bbb.70651. Epub 2008 Apr 7.

Abstract

5-Methylthioribulose-1-phosphate (MTRu-1-P) dehydratase catalyzes the reaction from MTRu-1-P to 2,3-diketo-5-methylthiopentyl-1-phosphate (DK-MTP-1-P) in the methionine salvage pathway in Bacillus subtilis. The properties of this enzyme remain to be determined. We characterized these properties using a recombinant protein. The enzyme, with a molecular mass of 90 kDa, was composed of four subunits. The K(m) and V(max) of the enzyme were 8.9 microM and 42.7 micromole min(-1) mg protein(-1) at 25 degrees C respectively. Maximum activity was observed at pH 7.5 to 8.5 and 40 degrees C. The activation energy of the reaction from MTRu-1-P to DK-MTP-1-P was 63.5 kJ mol(-1). The reaction product DK-MTP-1-P was labile, and decomposed at a rate constant of 0.048 s(-1) to an unknown compound that was not utilized by DK-MTP-1-P enolase, the enzyme catalyzing the next step. The function of this enzyme in the pathway is discussed.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Bacillus subtilis / enzymology*
  • Bacillus subtilis / metabolism
  • Hydro-Lyases / metabolism*
  • Hydrogen-Ion Concentration
  • Kinetics
  • Methionine / metabolism*
  • Phosphopyruvate Hydratase / metabolism
  • Ribulosephosphates / metabolism*
  • Temperature

Substances

  • Ribulosephosphates
  • 1-phospho-5-S-methylthioribulose
  • Methionine
  • Hydro-Lyases
  • Phosphopyruvate Hydratase