Singlet-triplet dispersion reveals additional frustration in the triangular-lattice dimer compound Ba3Mn2O8

Phys Rev Lett. 2008 Jun 13;100(23):237201. doi: 10.1103/PhysRevLett.100.237201. Epub 2008 Jun 9.

Abstract

We present single crystal inelastic neutron scattering measurements of the S=1 dimerized quasi-two-dimensional antiferromagnet Ba(3)Mn(2)O(8). The singlet-triplet dispersion reveals nearest-neighbor and next-nearest-neighbor ferromagnetic interactions between adjacent bilayers that compete against each other. Although the interbilayer exchange is comparable to the intrabilayer exchange, this additional frustration reduces the effective coupling along the c axis and leads to a quasi-two-dimensional behavior. In addition, the obtained exchange values are able to reproduce the four critical fields in the phase diagram.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.