Enhancement of somatostatin-receptor-targeted (177)Lu-[DOTA(0)-Tyr(3)]-octreotide therapy by gemcitabine pretreatment-mediated receptor uptake, up-regulation and cell cycle modulation

Nucl Med Biol. 2008 Aug;35(6):673-8. doi: 10.1016/j.nucmedbio.2008.05.003.

Abstract

Introduction: Clinical studies of patients treated with somatostatin-receptor (sstr)-targeted [DOTA(0)-Tyr(3)]-octreotide (DOTATOC) labeled with (177)Lu and (90)Y have shown overall response rates in the range of 9-33%. This study evaluates the potential for combination therapy with gemcitabine in an effort to improve clinical outcomes.

Methods: Human pancreatic adenocarcinoma Capan-2, rat pancreatic cancer AR42J and human small cell lung cancer NCI-H69 cells were each treated with 1 microg/ml gemcitabine for 4 days followed by replacement of the medium alone for four additional days. Cell cycle and direct receptor-uptake studies were performed with (177)Lu-DOTATOC after the total 8-day treatment as described. Cell viability and apoptosis experiments were performed to study the effects of gemcitabine pretreatment and (177)Lu-DOTATOC radionuclide therapy. Parallel control studies were performed with receptor-non-targeted (177)Lu-DOTA and DOTATOC.

Results: Cells treated with gemcitabine for 4 days showed a down-regulation of sstr expression as determined by (177)Lu-DOTATOC uptake. However, after 4 days of additional growth in absence of gemcitabine, the uptake of (177)Lu-DOTATOC was 1.5-3 times greater than that of the untreated control cells. In gemcitabine-pretreated Capan-2 cells, 84% of the cell population was in the G(2)M phase of the cell cycle. Due to sstr up-regulation and cell cycle modulations, synergistic effects of gemcitabine pretreatment were observed in cell viability and apoptosis assays. (177)Lu-DOTATOC resulted in two to three times greater apoptosis in gemcitabine-pretreated Capan-2 cells compared to the untreated cells.

Conclusion: Gemcitabine pretreatment up-regulates sstr expression and acts as a radiosensitizer through cell cycle modulation. The rational combination of gemcitabine and sstr-targeted radiopharmaceuticals represents a promising chemoradiation therapeutic tool with great potential to improve clinical outcomes and, thus, merits further study.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Antimetabolites, Antineoplastic / administration & dosage
  • Cell Cycle / drug effects
  • Cell Cycle / radiation effects*
  • Cell Line, Tumor
  • Cell Survival / drug effects
  • Cell Survival / radiation effects*
  • Deoxycytidine / administration & dosage
  • Deoxycytidine / analogs & derivatives*
  • Drug Delivery Systems / methods
  • Gemcitabine
  • Humans
  • Neoplasms / pathology*
  • Neoplasms / physiopathology*
  • Octreotide / administration & dosage
  • Octreotide / analogs & derivatives*
  • Octreotide / therapeutic use
  • Radiation-Sensitizing Agents / administration & dosage
  • Radiopharmaceuticals / administration & dosage*
  • Radiopharmaceuticals / therapeutic use
  • Receptors, Somatostatin / antagonists & inhibitors
  • Receptors, Somatostatin / radiation effects*
  • Up-Regulation / drug effects
  • Up-Regulation / radiation effects

Substances

  • 177Lu-octreotide, DOTA(0)-Tyr(3)-
  • Antimetabolites, Antineoplastic
  • Radiation-Sensitizing Agents
  • Radiopharmaceuticals
  • Receptors, Somatostatin
  • Deoxycytidine
  • Octreotide
  • Gemcitabine