Beta-lactoglobulin structure and retinol binding changes in presence of anionic and neutral detergents

J Agric Food Chem. 2008 Aug 27;56(16):7528-34. doi: 10.1021/jf801179k. Epub 2008 Aug 5.

Abstract

Bovine beta-lactoglobulin (beta-LG) in vivo (in milks) has been found in complexes with lipids such as butyric and oleic acids. To elucidate the still unknown structure-function relationship in this protein, the structural changes of beta-lactoglobulin variant A (beta-LG A) in the presence of anionic surfactant such as sodium n-dodecyl sulfate (SDS) and in the presence of nonionic surfactant such as Triton X-100 have been investigated. Subsequently, the retinol binding by beta-LG has been investigated in the presence of various amounts of these surfactants as its binding indicator. The results of UV-vis and fluorescence studies show a higher denaturating effect of SDS at acid pH that can be due to greater positive charges of beta-LG at this pH indicating also the nonspecific hydrophobic interactions of Triton X-100 with beta-LG at all studied pHs. Isothermal titration calorimetry (ITC) measurements indicate the endothermic nature of beta-LG/SDS interactions and the exothermic nature of Triton X-100/beta-LG interactions. The analysis of the binding data demonstrates the absence of considerable changes in retinol binding properties of beta-LG in the presence of various amounts of these surfactants. This implies that surfactant binding does not change the conformation of beta-LG in the regions defining the retinol-binding site.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Binding Sites
  • Calorimetry
  • Cattle
  • Detergents / pharmacology*
  • Lactoglobulins / chemistry*
  • Lactoglobulins / metabolism*
  • Molecular Structure
  • Octoxynol / pharmacology
  • Sodium Dodecyl Sulfate / pharmacology
  • Spectrometry, Fluorescence
  • Structure-Activity Relationship
  • Vitamin A / metabolism*

Substances

  • Detergents
  • Lactoglobulins
  • Vitamin A
  • Sodium Dodecyl Sulfate
  • Octoxynol