Mechanism of methaemoglobin breakdown by the lysine-specific gingipain of the periodontal pathogen Porphyromonas gingivalis

Biol Chem. 2008 Sep;389(9):1235-8. doi: 10.1515/BC.2008.140.

Abstract

Abstract The R- and K-gingipain proteases of Porphyromonas gingivalis are involved in proteolysis of haemoglobin from which the defensive dimeric haem pigment is formed. Whilst oxyhaemoglobin is refractory towards K-gingipain, methaemoglobin is rapidly degraded. Ligation of methaemoglobin with N3-, which effectively blocks haem dissociation from the protein, prevented haemoglobin breakdown. Haem-free globin was rapidly degraded by K-gingipain. These data emphasise the need for haemoglobin oxidation which encourages haem dissociation and makes the haem-free globin susceptible to proteolytic attack.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Adhesins, Bacterial / metabolism*
  • Animals
  • Cysteine Endopeptidases / metabolism*
  • Gingipain Cysteine Endopeptidases
  • Horses
  • Ligands
  • Methemoglobin / analogs & derivatives
  • Methemoglobin / metabolism*
  • Porphyromonas gingivalis / enzymology*

Substances

  • Adhesins, Bacterial
  • Gingipain Cysteine Endopeptidases
  • Ligands
  • methemoglobin azide
  • Methemoglobin
  • Cysteine Endopeptidases