Striking reactivity of ylide-like germylene toward terminal alkynes: [4+2] cycloaddition versus C-H bond activation

Chem Commun (Camb). 2008 Nov 14:(42):5393-5. doi: 10.1039/b811952j. Epub 2008 Sep 18.

Abstract

The isolable ylide-like N-heterocyclic germylene LGe: (2) {L = CH[(C=CH(2))CMe][N(aryl)](2), aryl = 2,6-(i)Pr(2)C(6)H(3)} shows an unprecedented dual reactivity toward terminal alkynes: its reaction with acetylene leads via [4+2] cycloaddition to the novel intramolecular donor stabilised germylene 3, while conversion of phenylacetylene furnishes the analogous cycloadduct 4 along with a C-H bond activation product, the novel N-donor stabilised alkynyl germylene 5.

MeSH terms

  • Alkynes / chemical synthesis*
  • Alkynes / chemistry
  • Computer Simulation
  • Crystallography, X-Ray
  • Cyclization
  • Germanium / chemistry*
  • Ligands
  • Models, Chemical
  • Models, Molecular
  • Molecular Structure
  • Organometallic Compounds / chemistry*

Substances

  • Alkynes
  • Ligands
  • Organometallic Compounds
  • Germanium