High-throughput experimentation platform: parallel microwave chemistry in HPLC/GC vials

J Comb Chem. 2009 May-Jun;11(3):460-8. doi: 10.1021/cc900007w.

Abstract

A high-throughput reaction platform for performing parallel microwave chemistry in sealed HPLC/GC vials is described. The system consists of a strongly microwave-absorbing silicon carbide plate with 20 cylindrical wells of appropriate dimensions to be fitted with standard HPLC/GC autosampler vials serving as reaction vessels. In combination with an aluminum sealing plate the setup can be used for microwave processing reaction volumes from 0.5-1.5 mL at a maximum temperature/pressure limit of 250 degrees C/20 bar. The parallel reaction platform displays excellent temperature and reaction homogeneity and has been used for high-throughput reaction optimization studies involving the parallel screening of catalyst, solvent and substrate reactivity for esterification reactions and metal-catalyzed dehydrative C-C couplings.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Carbon Compounds, Inorganic / chemistry*
  • Catalysis
  • Chromatography, Gas / instrumentation*
  • Chromatography, High Pressure Liquid / instrumentation*
  • Combinatorial Chemistry Techniques / economics
  • Combinatorial Chemistry Techniques / instrumentation*
  • Combinatorial Chemistry Techniques / methods*
  • Equipment Design / instrumentation
  • Hot Temperature
  • Microwaves
  • Pressure
  • Silicon Compounds / chemistry*
  • Solvents / chemistry
  • Substrate Specificity

Substances

  • Carbon Compounds, Inorganic
  • Silicon Compounds
  • Solvents
  • silicon carbide