Remarkable stabilization of M(12)L(24) spherical frameworks through the cooperation of 48 Pd(II)-pyridine interactions

J Am Chem Soc. 2009 May 6;131(17):6064-5. doi: 10.1021/ja900676f.

Abstract

Kinetic studies on the ligand exchange of self-assembled M(12)L(24) spherical complexes demonstrate that the multicomponent self-assembly roughly undergoes three stages. Initially, (i) there are very rapid equilibrations (ms(-1)) among the many components; (ii) as more stable structures are formed, the system equilibrates quickly (s(-1) to min(-1)) among the completed and uncompleted self-assemblies; misassembled structures are presumably corrected at this stage; and finally (iii) very slow equilibration (hours to days) at the final stage after the self-assembly completes, producing the kinetic stability of the whole. The half-lives of the ligand exchange processes in the M(12)L(24) complexes are much longer than those for comparable monodentate Pd(II)-pyridine complexes by a factor of approximately 10(5), suggesting that, once formed, the 36-component molecular spheres behave like covalent componds.

MeSH terms

  • Ligands
  • Magnetic Resonance Spectroscopy
  • Models, Molecular
  • Organometallic Compounds / chemistry*
  • Palladium / chemistry*
  • Pyridines / chemistry*

Substances

  • Ligands
  • Organometallic Compounds
  • Pyridines
  • Palladium