Combination of lacunary polyoxometalates and high-nuclear transition-metal clusters under hydrothermal conditions: first 6(5).8 cdSO4-type 3-D framework built by hexa-CuII sandwiched polyoxotungstates

Dalton Trans. 2009 Feb 28:(8):1300-6. doi: 10.1039/b809338e.

Abstract

A 6(5)8 CdSO4-type 3-D framework built by hexa-Cu" sandwiched polyoxotungstates [Cu(en)2]2-[Cu(deta)(H2O)]2[Cu6(en)2(H2O)2(B-alpha-GeW9O34)2] x 6H2O (1) (en = ethylenediamine and deta = diethylenetriamine) has been hydrothermally synthesized and structurally characterized by elemental analysis, IR spectrometry, thermogravimetric analysis and single-crystal X-ray diffraction. To the best of our knowledge, 1 represents the first 3-D TMSP with 6(5)-8 CdSO4 topology in polyoxometalate chemistry. Magnetic measurements performed on 1 indicate the occurrence of ferromagnetic interactions within the copper ions and the coupling constants can be determined.

MeSH terms

  • Crystallography, X-Ray
  • Electron Spin Resonance Spectroscopy
  • Magnetics
  • Metals / chemistry*
  • Models, Molecular
  • Spectrophotometry, Infrared
  • Sulfates / chemistry*
  • Tungsten / chemistry*

Substances

  • Metals
  • Sulfates
  • Tungsten