Metabolism of ticlopidine in rats: identification of the main biliary metabolite as a glutathione conjugate of ticlopidine S-oxide

Drug Metab Dispos. 2009 Sep;37(9):1904-15. doi: 10.1124/dmd.109.027524. Epub 2009 Jun 18.

Abstract

We have identified several novel metabolites of ticlopidine, a well known antiplatelet agent and have revealed its metabolic route in rats. The main biliary metabolite of ticlopidine was characterized as a glutathione (GSH) conjugate of ticlopidine S-oxide, in which conjugation had occurred at carbon 7a in the thienopyridine moiety. Quantitative analysis revealed that 29% of the dose was subjected to the formation of reactive intermediates followed by conjugation with GSH after oral administration of ticlopidine (22 mg/kg) to rats. In vitro incubation of ticlopidine with rat liver 9000 g supernatant fraction (S9) fractions led to the formation of multiple metabolites, including 2-oxo-ticlopidine, the precursor for the pharmacologically active ticlopidine metabolite, [1-(2-chlorobenzyl)-4-mercaptopiperidin-(3Z)-ylidene] acetic acid. A novel thiophene ring-opened metabolite with a thioketone group and a carboxylic acid moiety has also been detected after incubation of 2-oxo-ticlopidine with rat liver microsomes or upon incubation of ticlopidine with rat liver S9 fractions.

MeSH terms

  • Animals
  • Bile / metabolism*
  • Biotransformation
  • Chromatography, High Pressure Liquid
  • Fibrinolytic Agents / pharmacokinetics*
  • Fibrinolytic Agents / urine
  • Glutathione / metabolism*
  • Liver / metabolism
  • Magnetic Resonance Spectroscopy
  • Male
  • Mass Spectrometry
  • Microsomes, Liver / metabolism
  • Oxides / metabolism
  • Rats
  • Rats, Sprague-Dawley
  • Spectrophotometry, Ultraviolet
  • Subcellular Fractions / metabolism
  • Ticlopidine / pharmacokinetics*
  • Ticlopidine / urine

Substances

  • Fibrinolytic Agents
  • Oxides
  • Glutathione
  • Ticlopidine