On the mechanism of hydrogen peroxide formation during precipitation of hemoglobin with perchloric acid

Biol Chem Hoppe Seyler. 1990 Sep;371(9):881-7. doi: 10.1515/bchm3.1990.371.2.881.

Abstract

During acid precipitation of hemoglobin, hydrogen peroxide is formed. The oxidant is generated from hemoglobin-bound as well as from physically dissolved oxygen, provided divalent hemoglobin-iron is present. The extent of hydrogen peroxide formation seems to be dependent on the precipitating reagent. From experiments on GSH oxidation during precipitation of red cells and from a literature survey formation of at least one second reactive oxygen species has to be assumed. Different reaction pathways for generating these oxidants during acid precipitation are discussed: Hydroperoxide which is probably liberated by proton catalysis may contribute to the observed oxidation reactions. At pH approximately 1 it rapidly disproportionates yielding oxygen and hydrogen peroxide, which might produce reactive oxidants with hemoglobin intermediates formed during precipitation. In addition a new hypothesis is presented explaining the ability of N-ethylmaleimide to inhibit GSH oxidation during precipitation of red cells. Accordingly, the SH-reagent rapidly penetrates the cell membrane and reacts with GSH before access of protons prevents alkylation.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Chemical Precipitation
  • Glutathione / metabolism
  • Hemoglobins / metabolism*
  • Humans
  • Hydrogen Peroxide / metabolism*
  • Oxidation-Reduction
  • Oxygen / metabolism
  • Perchlorates / pharmacology*

Substances

  • Hemoglobins
  • Perchlorates
  • Hydrogen Peroxide
  • Glutathione
  • Oxygen