In vivo imaging of sentinel nodes using fluorescent silica nanoparticles in living mice

Mol Imaging Biol. 2010 Apr;12(2):155-62. doi: 10.1007/s11307-009-0262-8. Epub 2009 Oct 15.

Abstract

Purpose: We examine the feasibility of fluorescent imaging system for sentinel lymph node detection by using functionalized silica nanoparticles.

Materials and methods: We developed a functionalized RITC-SiO(2) nanoparticles containing fluorescent dye, C(28)H(31)N(2)O(3)Cl (rhodamine B isothiocyanate) inside, and subsequently synthesized (68)Ga-NOTA-RITC-SiO(2) nanoparticles.

Results: At 5 min after RITC-doped silica nanoparticles injection, fluorescent signals were shown in both right axillary lymph node (ALN) and injection site of living mice. Fluorescent signals were also observed at these locations in a biodistribution study. In addition, fluorescence was detected in frozen ALN sections microscopically. The percentages of doses injected per gram of tissue of axillary and brachial lymph nodes near footpad treated with (68)Ga-NOTA-RITC-SiO(2) nanoparticles were 308.3 +/- 3.4 and 41.5 +/- 6.1, respectively. Little (68)Ga radioactivity was found in other organs.

Conclusion: Our data provide strong evidence that functionalized silica nanoparticles has a promising potential as organic lymphatic tracer in biomedical imaging such as pre- and intraoperative surgical guidance.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Extremities
  • Female
  • Frozen Sections
  • Gallium / pharmacokinetics
  • Gallium / pharmacology
  • Heterocyclic Compounds / pharmacokinetics
  • Heterocyclic Compounds / pharmacology
  • Heterocyclic Compounds, 1-Ring
  • Lymph Nodes / anatomy & histology*
  • Lymph Nodes / drug effects*
  • Mice
  • Mice, Inbred BALB C
  • Microscopy, Fluorescence
  • Molecular Imaging / methods*
  • Nanoparticles / chemistry*
  • Nanoparticles / ultrastructure
  • Rhodamines / pharmacokinetics
  • Silicon Dioxide / pharmacokinetics
  • Silicon Dioxide / pharmacology*
  • Spectrometry, Fluorescence
  • Tissue Distribution / drug effects

Substances

  • Heterocyclic Compounds
  • Heterocyclic Compounds, 1-Ring
  • Rhodamines
  • 1,4,7-triazacyclononane-N,N',N''-triacetic acid
  • Silicon Dioxide
  • rhodamine isothiocyanate
  • Gallium