Detection of bright trion states using the fine structure emission of single CdSe/ZnS colloidal quantum dots

ACS Nano. 2009 Nov 24;3(11):3762-8. doi: 10.1021/nn9010158.

Abstract

We report direct observation of the lowest two states of the band-edge exciton fine structure in the photoluminescence from single CdSe/ZnS core/shell nanocrystals at cryogenic temperatures. The temperature dependence of this spectral fingerprint reveals exciton spin relaxation rates as low as 10 micros(-1). The fine structure is also dependent on the nanocrystal charge state facilitating the identification of a bright negatively charged trion state with a quantum yield comparable to that of neutral emission.

Publication types

  • Research Support, Non-U.S. Gov't