Ag/AgBr/WO(3).H(2)O: visible-light photocatalyst for bacteria destruction

Inorg Chem. 2009 Nov 16;48(22):10697-702. doi: 10.1021/ic9014652.

Abstract

A new composite photocatalyst Ag/AgBr/WO(3).H(2)O was synthesized by reacting Ag(8)W(4)O(16) with HBr and then reducing some Ag(+) ions in the surface region of AgBr particles to Ag nanoparticles via the light-induced chemical reduction. Ag nanoparticles are formed from AgBr by the light-induced chemical reduction reaction. The Ag/AgBr particles are on the surface of WO(3).H(2)O and have irregular shapes with sizes varying between 63 and 442 nm. WO(3).H(2)O appears as flakes about 31 nm thick and 157-474 nm wide. The as-grown Ag/AgBr/WO(3).H(2)O sample shows strong absorption in the visible region because of the plasmon resonance of Ag nanoparticles in Ag/AgBr/WO(3).H(2)O. The ability of this compound to destroy E. coli and oxidize methylic orange under visible light was compared with those of other reference photocatalysts. Ag/AgBr/WO(3).H(2)O is a highly efficient photocatalyst under visible light. The Ag/AgBr/WO(3).H(2)O samples recovered from repeated photooxidation experiments are almost identical to the as-prepared samples, proving the stability of Ag/AgBr/WO(3).H(2)O sample.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Azo Compounds / chemistry
  • Bromides / chemistry*
  • Catalysis
  • Crystallography, X-Ray
  • Escherichia coli / drug effects
  • Escherichia coli / metabolism*
  • Light*
  • Microscopy, Electron
  • Oxides / chemistry*
  • Oxides / metabolism
  • Oxides / pharmacology
  • Photochemical Processes*
  • Photoelectron Spectroscopy
  • Silver / chemistry*
  • Silver Compounds / chemistry*
  • Spectrophotometry, Ultraviolet
  • Tungsten / chemistry*
  • Tungsten / metabolism
  • Tungsten / pharmacology
  • Water / chemistry*

Substances

  • Azo Compounds
  • Bromides
  • Oxides
  • Silver Compounds
  • Water
  • Silver
  • methyl orange
  • tungsten oxide
  • silver bromide
  • Tungsten