Simultaneous quantitation of paracetamol, caffeine, pseudoephedrine, chlorpheniramine and cloperastine in human plasma by liquid chromatography-tandem mass spectrometry

J Pharm Biomed Anal. 2010 Feb 5;51(3):716-22. doi: 10.1016/j.jpba.2009.10.009. Epub 2009 Oct 14.

Abstract

A rapid and sensitive method based on liquid chromatography-tandem mass spectrometry (LC-MS/MS) for the simultaneous quantitation of paracetamol, caffeine, pseudoephedrine, chlorpheniramine and cloperastine in human plasma has been developed and validated. After sample preparation by liquid-liquid extraction, the analytes and internal standard (diphenhydramine) were analyzed by reversed-phase HPLC on a Venusil Mp-C(18) column (50mmx4.6mm, 5microm) using formic acid:10mM ammonium acetate:methanol (1:40:60, v/v/v) as mobile phase in a run time of 2.6min. Detection was carried out by electrospray positive ionization mass spectrometry in the multiple-reaction monitoring mode. The method was linear for all analytes over the following concentration (ng/ml) ranges: paracetamol 5.0-2000; caffeine 10-4000; pseudoephedrine 0.25-100; chlorpheniramine 0.05-20; cloperastine 0.10-40. Intra- and inter-day precisions (as relative standard deviation) were all < or =11.3% with accuracy (as relative error) of +/-5.0%. The method was successfully applied to a study of the pharmacokinetics of the five analytes after administration of a combination oral dose to healthy Chinese volunteers.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetaminophen / blood*
  • Caffeine / blood*
  • Chlorpheniramine / blood*
  • Chromatography, Liquid / methods
  • Evaluation Studies as Topic
  • Humans
  • Male
  • Piperidines / blood*
  • Pseudoephedrine / blood*
  • Tandem Mass Spectrometry / methods*

Substances

  • Piperidines
  • Acetaminophen
  • Caffeine
  • Chlorpheniramine
  • cloperastine
  • Pseudoephedrine