Immunochemical detection of rodent hepatic and urinary metabolites of cooking-induced food mutagens

Carcinogenesis. 1991 Feb;12(2):349-54. doi: 10.1093/carcin/12.2.349.

Abstract

Monoclonal antibodies, previously selected to bind either 2-amino-3,8-dimethylimidazo[4,5-f]quinoxaline (MeIQx) or 2-amino-1-methyl-6-phenylimidazo[4,5-b]pyridine (PhIP) were evaluated to determine their binding properties with several known metabolites of these compounds purified from rat hepatocyte cultures. Both 2-N- and 5-substituted MeIQx metabolites were recognized by antibodies AIA-2 and AIA-11, while antibodies AIA-1 and AIA-12 bound N-substituted metabolites only. Anti-PhIP antibodies bound N-hydroxy-PhIP, N-sulfinamide-glutathione-PhIP and N-hydroxy-glucuronide-PhIP. Immunoaffinity columns incorporating these antibodies were used to concentrate and purify both the unmetabolized parent compounds and several relatively non-polar metabolites from the urine of rats exposed either to MeIQx or PhIP. Several of these metabolites corresponded with available standards of previously identified polar conjugate metabolites, e.g. N-sulfamate-MeIQx and N(OH)-gluc-PhIP, while others are as yet unidentified. Immunoaffinity chromatography is demonstrated as a promising means of selectively concentrating metabolites of PhIP and MeIQx from urine.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Animals
  • Antibodies, Monoclonal / metabolism
  • Chromatography, Affinity
  • Food
  • Hot Temperature
  • Imidazoles / immunology
  • Imidazoles / metabolism*
  • Imidazoles / urine
  • Immunohistochemistry
  • Liver / metabolism*
  • Meat / toxicity*
  • Mutagens / metabolism*
  • Mutagens / urine
  • Quinolines / immunology
  • Quinolines / metabolism*
  • Quinolines / urine
  • Rats
  • Rats, Inbred F344

Substances

  • Antibodies, Monoclonal
  • Imidazoles
  • Mutagens
  • Quinolines
  • 2-amino-1-methyl-6-phenylimidazo(4,5-b)pyridine
  • 2-amino-3,4-dimethylimidazo(4,5-f)quinoline