Low-symmetry phases in ferroelectric nanowires

Nano Lett. 2010 Apr 14;10(4):1177-83. doi: 10.1021/nl9034708.

Abstract

Ferroelectric nanostructures have recently attracted much attention due to the quest of miniaturizing devices and discovering novel phenomena. In particular, studies conducted on two-dimensional and zero-dimensional ferroelectrics have revealed original properties and their dependences on mechanical and electrical boundary conditions. Meanwhile, researches aimed at discovering and understanding properties of one-dimensional ferroelectric nanostructures are scarce. The determination of the structural phase and of the direction of the polarization in one-dimensional ferroelectrics is of technological importance, since, e.g., a low-symmetry phase in which the polarization lies away from a highly symmetric direction typically generates phenomenal dielectric and electromechanical responses. Here, we investigate the phase transition sequence of nanowires made of KNbO(3) and BaTiO(3) perovskites, by combining X-ray diffraction, Raman spectroscopy, and first-principles-based calculations. We provide evidence of a previously unreported ferroelectric ground state of monoclinic symmetry and the tuning of the polarization's direction by varying factors inherent to the nanoscale.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Barium Compounds / chemistry*
  • Nanotechnology / methods*
  • Nanowires / chemistry*
  • Niobium / chemistry*
  • Oxides / chemistry*
  • Phase Transition
  • Potassium / chemistry*
  • Spectrum Analysis, Raman
  • Temperature
  • Titanium / chemistry*
  • X-Ray Diffraction

Substances

  • Barium Compounds
  • Oxides
  • Niobium
  • potassium niobate
  • barium titanate(IV)
  • Titanium
  • Potassium