Cochliones A-D, four new tetrahydrochromanone derivatives from endophytic Cochliobolus sp

J Asian Nat Prod Res. 2010 Jun;12(6):485-91. doi: 10.1080/10286020.2010.489819.

Abstract

Four new tetrahydrochromanone derivatives, cochliones A-D (1-4), along with three known metabolites, 4-hydroxybenzaldehyde (5), 4-hydroxy-3-(3-methylbut-2-enyl) benzoic acid (6), and 2,2-dimethyl-2H-chromene-6-carboxylic acid (7), were characterized from the culture of Cochliobolus sp. IFB-E039, a fungus that resides inside the healthy root of Cynodon dactylon (Gramineae). The structures of 1-4 were accommodated by their spectral data (UV, IR, CD, HR-ESI-MS, (1)H and (13)C NMR, (1)H-(1)H COSY, HMQC, HMBC, and NOESY). The bioassay for the cytotoxic metabolite showed that cochlione C (3) inhibited human breast adenocarcinoma cell line (MCF-7) and human chronic myeloid leukemia cell line (K562) with IC(50) values of 21.99 and 4.59 microg/ml, respectively.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antineoplastic Agents / chemistry
  • Antineoplastic Agents / isolation & purification*
  • Antineoplastic Agents / pharmacology
  • Ascomycota / chemistry*
  • China
  • Chromones / chemistry
  • Chromones / isolation & purification*
  • Chromones / pharmacology
  • Drug Screening Assays, Antitumor
  • Female
  • Hep G2 Cells
  • Humans
  • Inhibitory Concentration 50
  • K562 Cells
  • KB Cells
  • Molecular Structure
  • Nuclear Magnetic Resonance, Biomolecular

Substances

  • Antineoplastic Agents
  • Chromones