Total synthesis and stereochemical reassignment of tasiamide B

J Pept Sci. 2010 Jul;16(7):364-74. doi: 10.1002/psc.1254.

Abstract

The first total synthesis of tasiamide B, an octapeptide bearing 4-amino-3-hydroxy-5-phenylpentanoic acid unit isolated from the marine cyanobacteria Symploca sp. is described. A simple and efficient way was found to avoid the pyroglutamylation of N(alpha)-Me-Gln and led to a reassignment of the N(alpha)-Me-L-Phe of tasiamide B to be N(alpha)-Me-D-Phe, which was also supported by 1D and 2D NMR.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acids / chemistry
  • Cyanobacteria / chemistry
  • Magnetic Resonance Spectroscopy
  • Oligopeptides / chemical synthesis*
  • Oligopeptides / chemistry
  • Stereoisomerism

Substances

  • Amino Acids
  • Oligopeptides
  • tasiamide B
  • 4-amino-3-hydroxy-5-phenylpentanoic acid