The structure of cbb3 cytochrome oxidase provides insights into proton pumping

Science. 2010 Jul 16;329(5989):327-30. doi: 10.1126/science.1187303. Epub 2010 Jun 24.

Abstract

The heme-copper oxidases (HCOs) accomplish the key event of aerobic respiration; they couple O2 reduction and transmembrane proton pumping. To gain new insights into the still enigmatic process, we structurally characterized a C-family HCO--essential for the pathogenicity of many bacteria--that differs from the two other HCO families, A and B, that have been structurally analyzed. The x-ray structure of the C-family cbb3 oxidase from Pseudomonas stutzeri at 3.2 angstrom resolution shows an electron supply system different from families A and B. Like family-B HCOs, C HCOs have only one pathway, which conducts protons via an alternative tyrosine-histidine cross-link. Structural differences around hemes b and b3 suggest a different redox-driven proton-pumping mechanism and provide clues to explain the higher activity of family-C HCOs at low oxygen concentrations.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Catalytic Domain
  • Crystallography, X-Ray
  • Cytoplasm / metabolism
  • Electron Transport
  • Electron Transport Complex IV / chemistry*
  • Electron Transport Complex IV / metabolism*
  • Heme / chemistry
  • Histidine / chemistry
  • Hydrogen Bonding
  • Models, Molecular
  • Molecular Sequence Data
  • Oxidation-Reduction
  • Oxygen / metabolism
  • Periplasm / metabolism
  • Protein Conformation
  • Protein Structure, Secondary
  • Protein Structure, Tertiary
  • Proton Pumps / chemistry*
  • Proton Pumps / metabolism*
  • Protons*
  • Pseudomonas stutzeri / enzymology*
  • Tyrosine / chemistry

Substances

  • Proton Pumps
  • Protons
  • Tyrosine
  • Heme
  • Histidine
  • cbb3 oxidase
  • Electron Transport Complex IV
  • Oxygen

Associated data

  • GENBANK/HM130676
  • PDB/3MK7