Dosimetry of 18F-labeled tyrosine kinase inhibitor SKI-249380, a dasatinib-tracer for PET imaging

Mol Imaging Biol. 2012 Feb;14(1):25-31. doi: 10.1007/s11307-010-0462-2.

Abstract

Purpose: To obtain estimates of human normal-organ radiation doses of ¹⁸F-SKI-249380, as a prerequisite step towards first-in-human trial. ¹⁸F-SKI-249380 is a first-of-its-kind PET tracer for imaging the in vivo pharmacokinetics of dasatinib, an investigational targeted therapy for solid malignancies.

Procedures: Isoflurane-anesthetized mice received tracer dose via tail vein. Organ time-integrated activity coefficients, fractional urinary and hepatobiliary excretion, and total-body clearance kinetics were derived from PET data, with allometric extrapolation to the Standard Man anatomic model and normal-organ-absorbed dose calculations using OLINDA/EXM software.

Results: The human effective dose was 0.031 mSv/MBq. The critical organ was the upper large intestine, with a dose equivalent of 0.25 mSv/MBq. A 190-MBq administered activity of ¹⁸F-SKI-249380 is thus predicted to expose an adult human to radiation doses generally comparable to those of routinely used diagnostic radiopharmaceuticals.

Conclusions: Animal-based human dose estimates support first-in-human testing of ¹⁸F-SKI-249380.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Animals
  • Dasatinib
  • Female
  • Fluorine Radioisotopes / chemistry
  • Fluorine Radioisotopes / pharmacokinetics*
  • Male
  • Mice
  • Mice, Nude
  • Mice, SCID
  • Models, Animal
  • Molecular Imaging / methods*
  • Positron-Emission Tomography / methods*
  • Pyrimidines / chemistry
  • Pyrimidines / pharmacokinetics*
  • Radiation Dosage
  • Radiopharmaceuticals / chemistry
  • Radiopharmaceuticals / pharmacokinetics*
  • Thiazoles / chemistry
  • Thiazoles / pharmacokinetics*
  • Tissue Distribution

Substances

  • Fluorine Radioisotopes
  • Pyrimidines
  • Radiopharmaceuticals
  • Thiazoles
  • Dasatinib