Stereochemical nature of the products of linoleic acid oxidation catalyzed by lipoxygenases from potato and soybean

Biochem Biophys Res Commun. 1990 Jul 31;170(2):491-6. doi: 10.1016/0006-291x(90)92118-j.

Abstract

When linoleic acid was incubated with the purified potato lipoxygenase under O2 atmosphere, a mixture of 9 and 13-hydroperoxyoctadecadienoic acids was formed. Stereochemical analysis of the respective methyl-hydroxyoctadecadienoic acids revealed that the 9-isomer was in S-configuration whereas 13-hydroxyoctadecadienoic acid was a mixture of S (39%) and R (61%). Exactly the opposite was the case with the soybean lipoxygenase products, where the 13-isomer was found to be in S-configuration and 9-hydroxyoctadecadienoic acid - a mixture of S (73%) and R (27%). A general scheme is proposed for the stereochemical nature of oxidation products of enzymes which are predominantly either [+2] or [-2] lipoxygenases.

MeSH terms

  • Chromatography, High Pressure Liquid
  • Glycine max / enzymology*
  • Linoleic Acid
  • Linoleic Acids / metabolism*
  • Lipid Peroxides*
  • Lipoxygenase / metabolism*
  • Solanum tuberosum / enzymology*
  • Stereoisomerism

Substances

  • Linoleic Acids
  • Lipid Peroxides
  • 13-hydroperoxy-9,11-octadecadienoic acid
  • 9-hydroperoxy-11,12-octadecadienoic acid
  • Linoleic Acid
  • Lipoxygenase