First synthesis of C. difficile PS-II cell wall polysaccharide repeating unit

Org Lett. 2011 Feb 4;13(3):378-81. doi: 10.1021/ol1026188. Epub 2010 Dec 29.

Abstract

Clostridium difficile is the most commonly diagnosed cause of nosocomial diarrhea with increasing incidence and mortality among elderly and hospitalized patients. We report the first synthesis of the surface polysaccharide PS-II repeating unit and its nonphosphorylated analogue, with a linker for conjugation, via a (4 + 2) convergent approach from a common AB(D)C tetrasaccharide intermediate.

MeSH terms

  • Aged
  • Carbohydrate Sequence
  • Cell Wall / chemistry
  • Clostridioides difficile / chemistry*
  • Diarrhea / epidemiology*
  • Humans
  • Polysaccharides, Bacterial / chemistry*

Substances

  • Polysaccharides, Bacterial
  • polysaccharide II, Clostridium difficile