Structure based discovery of small molecule suppressors targeting bacterial lysozyme inhibitors

Biochem Biophys Res Commun. 2011 Feb 25;405(4):527-32. doi: 10.1016/j.bbrc.2011.01.053. Epub 2011 Jan 20.

Abstract

The production of lysozyme inhibitors, competitively binding to the lysozyme active site, is a bacterial strategy to prevent the lytic activity of host lysozymes. Therefore, suppression of the lysozyme-inhibitor interaction is an interesting new approach for drug development since restoration of the bacterial lysozyme sensitivity will support bacterial clearance from the infected sites. Using molecular modelling techniques the interaction of the Salmonella PliC inhibitor with c-type lysozyme was studied and a protein-protein interaction based pharmacophore model was created. This model was used as a query to identify molecules, with potential affinity for the target, and subsequently, these molecules were filtered using molecular docking. The retained molecules were validated as suppressors of lysozyme inhibitory proteins using in vitro experiments revealing four active molecules.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Anti-Bacterial Agents / chemistry*
  • Anti-Bacterial Agents / isolation & purification
  • Anti-Bacterial Agents / pharmacology
  • Bacterial Proteins / antagonists & inhibitors*
  • Bacterial Proteins / chemistry
  • Bacterial Proteins / metabolism
  • Computer Simulation
  • Drug Discovery / methods*
  • Models, Molecular*
  • Molecular Sequence Data
  • Muramidase / antagonists & inhibitors*
  • Muramidase / chemistry
  • Muramidase / metabolism
  • Protein Conformation
  • Recombinant Proteins / antagonists & inhibitors
  • Recombinant Proteins / chemistry
  • Recombinant Proteins / metabolism
  • Salmonella typhimurium / drug effects
  • Salmonella typhimurium / metabolism*

Substances

  • Anti-Bacterial Agents
  • Bacterial Proteins
  • Recombinant Proteins
  • Muramidase