Capture and activation of aerial CO2 by carbamoylation of L-threonine in a Ag(I) supramolecular framework

Dalton Trans. 2011 Jun 7;40(21):5677-9. doi: 10.1039/c1dt10571j. Epub 2011 Apr 21.

Abstract

An ultrasonic reaction of Ag(2)O, 4,4'-bipyridine (bipy) and (2S, 3R)-3-amino-2-hydroxybutanoic acid (L-Thr) gives an unexpected Ag(I) supramolecular framework, {[Ag(3)(bipy)(3)(cahba)]·HCO(3)·10H(2)O}(n) (1), in which the (2S, 3R)-3-(carboxyamino)-2-hydroxybutanoic acid (H(2)cahba) is a carbamate derivative of L-Thr, obtained via in situ transformation of amino group of L-Thr into carbamate by means of CO(2) uptake.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Carbamates / chemistry*
  • Carbon Dioxide / chemistry*
  • Oxides / chemistry*
  • Pyridines / chemistry
  • Silver Compounds / chemistry*
  • Stereoisomerism
  • Threonine / chemistry*
  • Ultrasonics

Substances

  • Carbamates
  • Oxides
  • Pyridines
  • Silver Compounds
  • Carbon Dioxide
  • Threonine
  • disilver oxide
  • 4,4'-bipyridyl