Choice of biological source material supersedes oxidative stress in its influence on DJ-1 in vivo interactions with Hsp90

J Proteome Res. 2011 Oct 7;10(10):4388-404. doi: 10.1021/pr200225c. Epub 2011 Aug 26.

Abstract

DJ-1 is a small but relatively abundant protein of unknown function that may undergo stress-dependent cellular translocation and has been implicated in both neurodegenerative diseases and cancer. As such, DJ-1 may be an excellent study object to elucidate the relative influence of the cellular context on its interactome and for exploring whether acute exposure to oxidative stressors alters its molecular environment. Using quantitative mass spectrometry, we conducted comparative DJ-1 interactome analyses from in vivo cross-linked brains or livers and from hydrogen peroxide-treated or naïve embryonic stem cells. The analysis identified a subset of glycolytic enzymes, heat shock proteins 70 and 90, and peroxiredoxins as interactors of DJ-1. Consistent with a role of DJ-1 in Hsp90 chaperone biology, we document destabilization of Hsp90 clients in DJ-1 knockout cells. We further demonstrate the existence of a C106 sulfinic acid modification within DJ-1 and thereby establish that this previously inferred modification also exists in vivo. Our data suggest that caution has to be exerted in interpreting interactome data obtained from a single biological source material and identify a role of DJ-1 as an oxidative stress sensor and partner of a molecular machinery notorious for its involvement in cell fate decisions.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cysteine / chemistry
  • Gene Expression Regulation, Neoplastic*
  • HSC70 Heat-Shock Proteins / metabolism
  • HSP90 Heat-Shock Proteins / metabolism*
  • Humans
  • Intracellular Signaling Peptides and Proteins / metabolism*
  • Mass Spectrometry / methods
  • Mice
  • Mice, Knockout
  • Oncogene Proteins / metabolism*
  • Oxidative Stress*
  • Peroxiredoxins / chemistry
  • Protein Deglycase DJ-1
  • Proteome
  • Proteomics / methods*
  • Sulfinic Acids / chemistry

Substances

  • HSC70 Heat-Shock Proteins
  • HSP90 Heat-Shock Proteins
  • Intracellular Signaling Peptides and Proteins
  • Oncogene Proteins
  • Proteome
  • Sulfinic Acids
  • Peroxiredoxins
  • PARK7 protein, human
  • PARK7 protein, mouse
  • Protein Deglycase DJ-1
  • Cysteine