Therapeutic potential of pegylated hemin for reactive oxygen species-related diseases via induction of heme oxygenase-1: results from a rat hepatic ischemia/reperfusion injury model

J Pharmacol Exp Ther. 2011 Dec;339(3):779-89. doi: 10.1124/jpet.111.185348. Epub 2011 Sep 2.

Abstract

Many diseases and pathological conditions, including ischemia/reperfusion (I/R) injury, are the consequence of the actions of reactive oxygen species (ROS). Controlling ROS generation or its level may thus hold promise as a standard therapeutic modality for ROS-related diseases. Here, we assessed heme oxygenase-1 (HO-1), which is a crucial antioxidative, antiapoptotic molecule against intracellular stresses, for its therapeutic potential via its inducer, hemin. To improve the solubility and in vivo pharmacokinetics of hemin for clinical applications, we developed a micellar hemin by conjugating it with poly(ethylene glycol) (PEG) (PEG-hemin). PEG-hemin showed higher solubility in water and significantly prolonged plasma half-life than free hemin, which resulted from its micellar nature with molecular mass of 126 kDa in aqueous media. In a rat I/R model, administration of PEG-hemin significantly elevated HO-1 expression and enzymatic activity. This induction of HO-1 led to significantly improved liver function, reduced apoptosis and thiobarbituric acid reactive substances of the liver, and decreased inflammatory cytokine production. PEG-hemin administration also markedly improved hepatic blood flow. These results suggest that PEG-hemin exerted a significant cytoprotective effect against I/R injury in rat liver by inducing HO-1 and thus seems to be a potential therapeutic for ROS-related diseases, including I/R injury.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Apoptosis / drug effects
  • Carbon Monoxide / blood
  • Cardiotonic Agents / pharmacology*
  • Caspase 3 / metabolism
  • Caspase 7 / metabolism
  • Cell Survival / drug effects
  • Chemokine CCL2 / blood
  • Disease Models, Animal
  • Dose-Response Relationship, Drug
  • Drug Evaluation, Preclinical
  • Enzyme Induction
  • Heme Oxygenase-1 / biosynthesis*
  • Hemin / analogs & derivatives*
  • Hemin / chemistry
  • Hemin / pharmacology
  • Hemin / therapeutic use*
  • Hepatocytes / drug effects
  • Humans
  • Liver / drug effects
  • Liver / metabolism*
  • Liver Circulation
  • Liver Diseases / drug therapy*
  • Liver Diseases / metabolism
  • Liver Diseases / physiopathology
  • Male
  • Polyethylene Glycols / chemistry
  • Polyethylene Glycols / pharmacology
  • Polyethylene Glycols / therapeutic use*
  • Rats
  • Rats, Wistar
  • Reactive Oxygen Species / metabolism*
  • Reperfusion Injury / drug therapy*
  • Reperfusion Injury / metabolism
  • Reperfusion Injury / physiopathology
  • Transaminases / blood

Substances

  • Cardiotonic Agents
  • Chemokine CCL2
  • Reactive Oxygen Species
  • Polyethylene Glycols
  • Hemin
  • Carbon Monoxide
  • Heme Oxygenase-1
  • Transaminases
  • Caspase 3
  • Caspase 7