Spin waves and magnetic exchange interactions in insulating Rb(0.89)Fe(1.58)Se(2)

Nat Commun. 2011 Dec 6:2:580. doi: 10.1038/ncomms1573.

Abstract

The parent compounds of iron pnictide superconductors are bad metals with a collinear antiferromagnetic structure and Néel temperatures below 220 K. Although alkaline iron selenide A(y)Fe(1.6+x)Se(2) (A=K, Rb, Cs) superconductors are isostructural with iron pnictides, in the vicinity of the undoped limit they are insulators, forming a block antiferromagnetic order and having Néel temperatures of roughly 500 K. Here we show that the spin waves of the insulating antiferromagnet Rb(0.89)Fe(1.58)Se(2) can be accurately described by a local moment Heisenberg Hamiltonian. A fitting analysis of the spin wave spectra reveals that the next-nearest neighbour couplings in Rb(0.89)Fe(1.58)Se(2), (Ba,Ca,Sr)Fe(2)As(2), and Fe(1.05)Te are of similar magnitude. Our results suggest a common origin for the magnetism of all the Fe-based superconductors, despite having different ground states and antiferromagnetic orderings.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Chemistry, Physical*
  • Crystallography, X-Ray
  • Electric Conductivity
  • Electrons
  • Ferrous Compounds / chemistry*
  • Iron / chemistry*
  • Magnetics / methods*
  • Molecular Structure
  • Rubidium / chemistry
  • Selenium / chemistry
  • Temperature
  • Thermodynamics

Substances

  • Ferrous Compounds
  • Iron
  • Selenium
  • Rubidium