Direct, regioselective, and chemoselective preparation of novel boronated tryptophans by Friedel-Crafts alkylation

Org Lett. 2012 Jan 20;14(2):600-3. doi: 10.1021/ol203216h. Epub 2011 Dec 30.

Abstract

A facile synthetic approach to the direct preparation of various novel unnatural boronated protected tryptophans using a regio- and chemoselective electrophilic substitution of 4- and 5-boronated indoles with N-protected dehydroalanine is described. The gram-scale synthesis of two free tryptophan boronic acids is also reported.

MeSH terms

  • Alkylation
  • Bromine Compounds / chemistry*
  • Hydrolysis
  • Molecular Structure
  • Stereoisomerism
  • Tryptophan / chemistry*

Substances

  • Bromine Compounds
  • Tryptophan