Hydroxyl radical generation mechanism during the redox cycling process of 1,4-naphthoquinone

Environ Sci Technol. 2012 Mar 6;46(5):2935-42. doi: 10.1021/es203032v. Epub 2012 Feb 22.

Abstract

Airborne quinones contribute to adverse health effects of ambient particles probably because of their ability to generate hydroxyl radicals (·OH) via redox cycling, but the mechanisms remain unclear. We examined the chemical mechanisms through which 1,4-naphthoquinone (1,4-NQ) induced ·OH, and the redox interactions between 1,4-NQ and ascorbate acid (AscH(2)). First, ·OH formation by 1,4-NQ was observed in cellular and acellular systems, and was enhanced by AscH(2). AscH(2) also exacerbated the cytotoxicity of 1,4-NQ in Ana-1 macrophages, at least partially due to enhanced ·OH generation. The detailed mechanism was studied in an AscH(2)/H(2)O(2) physiological system. The existence of a cyclic 1,4-NQ process was shown by detecting the corresponding semiquinone radical (NSQ·-) and hydroquinone (NQH(2)). 1,4-NQ was reduced primarily to NSQ·- by O2·- (which was from AscH(2) reacting with H(2)O(2)), not by AscH(2) as normally thought. At lower doses, 1,4-NQ consumed O2·- to suppress ·OH; however, at higher doses, 1,4-NQ presented a positive association with ·OH. The reaction of NSQ·- with H(2)O(2) to release ·OH was another important channel for OH radical formation except for Haber-Weiss reaction. As a reaction precursor for O2·-, the enhanced ·OH response to 1,4-NQ by AscH(2) was indirect. Reducing substrates were necessary to sustain the redox cycling of 1,4-NQ, leading to more ·OH and a deleterious end point.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Ascorbic Acid / pharmacology
  • Benzoquinones / chemistry
  • Cell Death / drug effects
  • Cell Line
  • Electron Spin Resonance Spectroscopy
  • Hydroxyl Radical / chemistry*
  • Macrophages / cytology
  • Macrophages / drug effects
  • Mice
  • Models, Biological
  • Naphthoquinones / chemistry*
  • Naphthoquinones / toxicity
  • Oxidation-Reduction / drug effects

Substances

  • Benzoquinones
  • Naphthoquinones
  • semiquinone radicals
  • Hydroxyl Radical
  • Ascorbic Acid
  • 1,4-naphthoquinone