Discovery of a new class of ghrelin receptor antagonists

Bioorg Med Chem Lett. 2012 Mar 1;22(5):2046-51. doi: 10.1016/j.bmcl.2012.01.014. Epub 2012 Jan 14.

Abstract

A series of benzodiazepine antagonists of the human ghrelin receptor GHSR1a were synthesized and their antagonism and metabolic stability were evaluated. The potency of these analogs was determined using a functional aequorin (Euroscreen) luminescent assay measuring the intracellular Ca(2+) concentration, and their metabolic stability was measured using an in vitro rat and human S9 hepatocyte assay. These efforts led to the discovery of a potent ghrelin antagonist with good rat pharmacokinetic properties.

MeSH terms

  • Animals
  • Benzodiazepines / chemistry*
  • Benzodiazepines / metabolism
  • Benzodiazepines / pharmacokinetics
  • Benzodiazepines / pharmacology*
  • Calcium / metabolism
  • Cell Line
  • Hepatocytes / metabolism
  • Humans
  • Luminescent Measurements
  • Obesity / drug therapy
  • Rats
  • Rats, Sprague-Dawley
  • Receptors, Ghrelin / antagonists & inhibitors*
  • Receptors, Ghrelin / metabolism*
  • Structure-Activity Relationship

Substances

  • Receptors, Ghrelin
  • Benzodiazepines
  • Calcium