Acyl and silyl group effects in reactivity-based one-pot glycosylation: synthesis of embryonic stem cell surface carbohydrates Lc4 and IV(2)Fuc-Lc4

J Am Chem Soc. 2012 Mar 14;134(10):4549-52. doi: 10.1021/ja300284x. Epub 2012 Mar 5.

Abstract

Relative reactivity evaluations showed the graded arming of toluenyl thioglucosides by variously positioned silyl groups but not by their acyl counterparts. These findings were applied in reactivity-based one-pot assembly of linker-attached Lc(4) and IV(2)Fuc-Lc(4), which are components of human embryonic stem cell surface. The sugar-galectin-1 binding was also examined.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Carbohydrate Sequence
  • Embryonic Stem Cells / chemistry*
  • Fucose / chemistry*
  • Glycosylation
  • Molecular Sequence Data

Substances

  • Fucose