Ynamides: stable ligand equivalents of unstable oxazol-4-ylidenes (novel mesoionic carbenes)

Chem Commun (Camb). 2012 Jul 18;48(56):7088-90. doi: 10.1039/c2cc33319h. Epub 2012 Jun 11.

Abstract

Deprotonation of an oxazolium salt induces a ring opening process leading to the corresponding ynamide. Although the expected mesoionic carbene is not obtained, the acyclic ynamide readily reacts with various transition metals yielding robust mesoionic carbene complexes.