A triptycene-based approach to solubilising carbon nanotubes and C60

Chemistry. 2012 Jul 9;18(28):8716-23. doi: 10.1002/chem.201101189. Epub 2012 Jun 12.

Abstract

We describe herein the synthesis of a triptycene-based surfactant designed with the ability to solubilise single-walled carbon nanotubes (SWNTs) and C(60) in water through non-covalent interactions. Furthermore, an amphiphilic naphthalene-based surfactant with the same ability to solubilise SWNTs and C(60) has also been prepared. The compounds synthesised were designed with either two ionic or non-ionic tails to ensure a large number of supramolecular interactions with the solvent, thereby promoting strong solubilisation. The surfactants produced stable suspensions in which the SWNTs are dispersed and the surfactant/SWNT complexes formed are stable for more than one year. UV/Vis/NIR absorption spectroscopy, TEM and AFM were employed to probe the solubilisation properties of the dispersion of surfactants and SWNTs in water.

MeSH terms

  • Anthracenes / chemistry*
  • Fullerenes / chemistry*
  • Molecular Structure
  • Nanotubes, Carbon / chemistry*
  • Solubility
  • Spectroscopy, Near-Infrared
  • Surface-Active Agents / chemistry
  • Water / chemistry

Substances

  • Anthracenes
  • Fullerenes
  • Nanotubes, Carbon
  • Surface-Active Agents
  • Water
  • triptycene
  • fullerene C60