An historic perspective of proteasome inhibition

Semin Hematol. 2012 Jul;49(3):196-206. doi: 10.1053/j.seminhematol.2012.04.009.

Abstract

The ubiquitin-proteasome system (UPS) and associated signaling pathways are regarded today as an exciting area of development for novel therapeutics. However, two decades ago, following the discovery and elucidation of ubiquitin and the 26S proteasome as key mediators of protein turnover, the concept of inhibiting the UPS was not even considered a feasible therapeutic approach due to the assumption that inhibition of this pathway would have widespread deleterious effects. Subsequent clinical developments with the first-in-class proteasome inhibitor bortezomib have radically overturned that view, with the proteasome now recognized as a validated target and proteasome inhibition demonstrated to be a highly successful treatment for a number of hematologic malignancies. Here we provide a historic perspective on the emergence of proteasome inhibition, sharing some of the lessons learned along the way. We describe the development of bortezomib and the elucidation of the effects of its novel mechanism of action, and place the cutting-edge work described elsewhere in this issue in the context of these historic developments.

Publication types

  • Historical Article
  • Research Support, Non-U.S. Gov't
  • Review

MeSH terms

  • Animals
  • Antineoplastic Agents / history*
  • Antineoplastic Agents / pharmacology
  • Antineoplastic Agents / therapeutic use
  • Boronic Acids / history*
  • Boronic Acids / pharmacology
  • Boronic Acids / therapeutic use
  • Bortezomib
  • Drug Screening Assays, Antitumor
  • Hematologic Neoplasms / drug therapy
  • Hematologic Neoplasms / metabolism
  • History, 20th Century
  • History, 21st Century
  • Humans
  • Proteasome Endopeptidase Complex / history*
  • Proteasome Endopeptidase Complex / metabolism
  • Proteasome Inhibitors / history*
  • Proteasome Inhibitors / pharmacology
  • Proteasome Inhibitors / therapeutic use
  • Pyrazines / history*
  • Pyrazines / pharmacology
  • Pyrazines / therapeutic use
  • Structure-Activity Relationship
  • Ubiquitin / antagonists & inhibitors
  • Ubiquitin / history
  • Ubiquitin / metabolism

Substances

  • Antineoplastic Agents
  • Boronic Acids
  • Proteasome Inhibitors
  • Pyrazines
  • Ubiquitin
  • Bortezomib
  • Proteasome Endopeptidase Complex