From "loose" to "dense" crystalline phases of calcium carbonate through "repulsive" interactions: an experimental charge-density study

Chemistry. 2012 Oct 1;18(40):12633-6. doi: 10.1002/chem.201201457. Epub 2012 Aug 22.

Abstract

Anion-anion interactions in an eggshell: experimental electron density analysis for two polymorphs of calcium carbonate revealed why the less stable form, aragonite, has higher density than the most stable form, calcite. Although believed to be exclusively repulsive, the interactions between anions cause them to bind more tightly in a crystal and thus make the aragonite phase denser than its calcite counterpart.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Anions / chemistry*
  • Calcium Carbonate / chemistry*
  • Crystallography, X-Ray
  • Egg Shell / chemistry*
  • Egg Shell / metabolism*
  • Quantum Theory

Substances

  • Anions
  • Calcium Carbonate