Determinants of the essential one-carbon metabolism metabolites, homocysteine, S-adenosylmethionine, S-adenosylhomocysteine and folate, in cerebrospinal fluid

Clin Chem Lab Med. 2012 Mar 24;50(9):1641-7. doi: 10.1515/cclm-2012-0056.

Abstract

Background: Disturbances in the levels of one-carbon (1C) metabolism metabolites have been associated with a wide variety of neuropsychiatric diseases. Cerebrospinal fluid (CSF) levels of homocysteine (Hcy) and the other 1C metabolites, nor their interrelatedness and putative determinants, have been studied extensively in a healthy population.

Methods: Plasma and CSF samples from 100 individuals free from neuropsychiatric diseases were analyzed (55 male, 45 female; age 50±17 years). In blood, we measured plasma Hcy, serum folate and serum vitamin B12. In CSF, we measured total Hcy, S-adenosylmethionine (SAM), S-adenosylhomocysteine (SAH) and 5-methyltetrahydrofolate (5-methylTHF). Highly selective analytical methods like liquid chromatography combined with either mass spectrometry or fluorescence detection were used.

Results: CSF Hcy was inversely correlated with CSF 5-methylTHF and positively with plasma Hcy, independent of serum folate status. CSF SAH correlated with age, lower CSF 5-methylTHF and higher CSF Hcy. CSF 5-methylTHF showed independent negative correlations with age and positive correlations with serum folate. CSF SAM did not correlate with any of the 1C metabolites.

Conclusions: Aging is characterized by a reduction in CSF 5-methylTHF levels and increased CSF levels of the potentially neurotoxic transmethylation inhibitor SAH. CSF 5-methylTHF, which is itself determined in part by systemic folate status, is a powerful independent determinant of CSF levels of Hcy and SAH.

MeSH terms

  • Adult
  • Aged
  • Aging
  • Chromatography, High Pressure Liquid
  • Female
  • Folic Acid / blood
  • Folic Acid / cerebrospinal fluid*
  • Homocysteine / cerebrospinal fluid*
  • Humans
  • Immunoassay
  • Male
  • Middle Aged
  • S-Adenosylhomocysteine / cerebrospinal fluid*
  • S-Adenosylmethionine / cerebrospinal fluid*
  • Tandem Mass Spectrometry
  • Vitamin B 12 / blood

Substances

  • Homocysteine
  • S-Adenosylmethionine
  • Folic Acid
  • S-Adenosylhomocysteine
  • Vitamin B 12