New technology for transmission measurements in process pipes

Appl Radiat Isot. 2013 Feb:72:89-95. doi: 10.1016/j.apradiso.2012.10.005. Epub 2012 Oct 17.

Abstract

Transmission measurements of radiation through process pipes provide a non-intrusive method of determining the amount of product present in the pipes. The product could be a liquid, a slurry, or a gas, which is the most challenging because of the low density. Traditionally, these techniques have used a radioactive source that has to be replaced periodically. We have developed a transmission technique based on an X-ray tube instead of a decaying source. A notch filter is used to provide a narrow transmission line, and a thin silicon transmission detector is used to monitor the X-ray tube output. The transmitted X-rays are measured with a high-throughput gamma spectrometer that consists of a NaI(Tl) detector and an MCA with precise dead time correction. This spectrometer provides stable transmission measurements with an accuracy of a fraction of a percent. The shielding and collimator are made of machinable tungsten for thermal mechanical stability, as well low-cost, low-weight tungsten powder in polymer castings. We describe two methods of measuring the pipe wall thickness without evacuating the pipe. Our particular application was for enrichment monitors for UF(6) in process pipes. Enrichment monitors that are independent of the plant data require two measurements: a transmission measurement to determine the total amount of uranium in the pipe and a measurement of the 186-keV gamma-ray line to determine the amount of (235)U present. The ratio of these values gives the enrichment. Previous designs used a decaying radioactive source such as (57)Co (122 keV, T(½)=272 days) or (109)Cd (22 keV, T(½)=1.2 years). A major effort was required to access and periodically replace these sources in operating plants. In this report, we describe the use of an X-ray tube, which eliminated the source problem, and other innovations. Then we present data from an enrichment monitor that incorporates these innovations.