[Preparation and in vitro properties of folate receptor targeting docetaxel-loaded amphiphilic copolymer-modified liposomes]

Yao Xue Xue Bao. 2012 Sep;47(9):1219-26.
[Article in Chinese]

Abstract

A novel amphiphilic copolymer, folate-poly (PEG-cyanoacrylate-co-cholesteryl cyanoacrylate) (FA-PEG-PCHL) was synthesized as liposomal modifying material with folate receptor targeting and long circulating property. FA-PEG-PCHL-modified docetaxel-loaded liposomes (FA-PDCT-L) were prepared by organic solvent injection method, and the system was optimized using central composite design-response surface methodology. The structure of the FA-PEG-PCHL copolymer was confirmed by FT-IR and 1H NMR. Ultrafiltration technique, transmission electron microscope, dynamic light scattering and electrophoretic light scattering, and fluorescence polarization method were used to study the physicochemical parameters of FA-PDCT-L. FA-PDCT-L showed spherical or ellipsoid shape. The mean particle sizes were in the range of 111.6-126.9 nm, zeta potentials were from -6.54 mV to -14.13 mV and the drug encapsulation efficiency achieved 97.8%. The observed values agreed well with model predicted values. The membrane fluidity increased with the increment of the molecular weight of PEG and the decrement of the amount of FA-PEG-PCHL. The in vitro release test showed that the drug could be sustained-released from liposomes without a burst release and with stability for 6 months. After 24 h only 31.1%, 27.2% and 19.5% of encapsulated docetaxel were released for FA-PDCT10000-L, FA-PDCT4000-L and FA-PDCT2000-L, respectively. This work is useful for further research on the application of the synthesized copolymer-modified long circulating liposomes for cancer therapy.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antineoplastic Agents / administration & dosage*
  • Cholesterol Esters / chemistry
  • Cyanoacrylates / chemistry
  • Delayed-Action Preparations
  • Docetaxel
  • Drug Carriers / chemical synthesis*
  • Drug Carriers / chemistry
  • Drug Delivery Systems*
  • Folate Receptors, GPI-Anchored / chemistry
  • Liposomes / administration & dosage
  • Liposomes / chemistry
  • Molecular Weight
  • Particle Size
  • Polyethylene Glycols / chemistry
  • Polymers / chemical synthesis
  • Polymers / chemistry
  • Taxoids / administration & dosage*

Substances

  • Antineoplastic Agents
  • Cholesterol Esters
  • Cyanoacrylates
  • Delayed-Action Preparations
  • Drug Carriers
  • Folate Receptors, GPI-Anchored
  • Liposomes
  • Polymers
  • Taxoids
  • Docetaxel
  • Polyethylene Glycols