First examples of metal-organic frameworks with the novel 3,3'-(1,2,4,5-tetrazine-3,6-diyl)dibenzoic spacer. Luminescence and adsorption properties

Inorg Chem. 2013 Jan 18;52(2):546-8. doi: 10.1021/ic302318j. Epub 2013 Jan 3.

Abstract

We report the synthesis of a novel ligand, 3,3'-(1,2,4,5-tetrazine-3,6-diyl)dibenzoic acid (1). In this fragment, we have introduced two carboxylate groups with the aim of using this ligand as a linker to construct three-dimensional metal-organic frameworks (MOFs). We have been successful in the formation of zinc (2) and lanthanum (3) MOFs. The zinc compound is a two-dimensional structure, while the lanthanum material is a three-dimensional MOF with interesting channels. We include the luminescence and adsorption studies of these materials. Moreover, we have evaluated the in vitro toxicity of this novel ligand, concluding that it can be considered negligible.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Adsorption
  • Animals
  • Benzoates / chemical synthesis*
  • Benzoates / chemistry
  • Cell Survival
  • Cells, Cultured
  • Crystallography, X-Ray
  • Heterocyclic Compounds / chemical synthesis*
  • Heterocyclic Compounds / chemistry
  • Humans
  • Lanthanum / chemistry
  • Luminescence
  • Organometallic Compounds / chemical synthesis*
  • Organometallic Compounds / chemistry
  • Organometallic Compounds / metabolism
  • Zinc / chemistry

Substances

  • 3,3'-(1,2,4,5-tetrazine-3,6-diyl)dibenzoic acid
  • Benzoates
  • Heterocyclic Compounds
  • Organometallic Compounds
  • Lanthanum
  • Zinc