29Si-1H IMPACT HMBC: a suitable tool for analyzing silylated derivatives

Magn Reson Chem. 2013 Apr;51(4):230-3. doi: 10.1002/mrc.3932. Epub 2013 Feb 13.

Abstract

A modified version of the IMPACT heteronuclear multiple bond correlation (HMBC) has allowed the characterization of an organosilane and a tetrasilylated yttrium complex. With the help of this sequence, an average gain in sensitivity close to 2 has been obtained compared with the standard HMBC experiment for disilanes as well as for yttrium complexes containing silylated ligands. This modified version of this long-range correlation experiment opens the way for following kinetics in the range of a fraction of a minute and to study by NMR low concentrated samples and low abundant nuclei.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Isotopes / chemistry
  • Magnetic Resonance Spectroscopy / standards
  • Molecular Structure
  • Organometallic Compounds / analysis*
  • Organometallic Compounds / chemical synthesis
  • Organosilicon Compounds / analysis*
  • Organosilicon Compounds / chemical synthesis
  • Protons
  • Reference Standards
  • Silicon / chemistry*

Substances

  • Isotopes
  • Organometallic Compounds
  • Organosilicon Compounds
  • Protons
  • Silicon