Structure of Pseudomonas aeruginosa inosine 5'-monophosphate dehydrogenase

Acta Crystallogr Sect F Struct Biol Cryst Commun. 2013 Mar 1;69(Pt 3):243-7. doi: 10.1107/S1744309113002352. Epub 2013 Feb 22.

Abstract

Inosine 5'-monophosphate dehydrogenase (IMPDH) represents a potential antimicrobial drug target. The crystal structure of recombinant Pseudomonas aeruginosa IMPDH has been determined to a resolution of 2.25 Å. The structure is a homotetramer of subunits dominated by a (β/α)8-barrel fold, consistent with other known structures of IMPDH. Also in common with previous work, the cystathionine β-synthase domains, residues 92-204, are not present in the model owing to disorder. However, unlike the majority of available structures, clearly defined electron density exists for a loop that creates part of the active site. This loop, composed of residues 297-315, links α8 and β9 and carries the catalytic Cys304. P. aeruginosa IMPDH shares a high level of sequence identity with bacterial and protozoan homologues, with residues involved in binding substrate and the NAD+ cofactor being conserved. Specific differences that have been proven to contribute to selectivity against the human enzyme in a study of Cryptosporidium parvum IMPDH are also conserved, highlighting the potential value of IMPDH as a drug target.

Keywords: Pseudomonas aeruginosa; antimicrobial drug targets; inosine 5′-monophosphate dehydrogenase.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Bacterial Proteins / chemistry*
  • Bacterial Proteins / genetics
  • Catalytic Domain
  • Conserved Sequence
  • Cryptosporidium parvum / chemistry
  • Cryptosporidium parvum / metabolism
  • Crystallography, X-Ray
  • Cysteine / chemistry*
  • Cysteine / genetics
  • Escherichia coli / chemistry
  • Escherichia coli / genetics
  • IMP Dehydrogenase / chemistry*
  • IMP Dehydrogenase / genetics
  • Models, Molecular
  • Molecular Sequence Data
  • Protein Multimerization
  • Protein Structure, Secondary
  • Protein Structure, Tertiary
  • Pseudomonas aeruginosa / chemistry*
  • Pseudomonas aeruginosa / enzymology
  • Sequence Alignment
  • Sequence Homology, Amino Acid
  • Species Specificity

Substances

  • Bacterial Proteins
  • IMP Dehydrogenase
  • Cysteine

Associated data

  • PDB/3ZFH