N-formylation of amines by methanol activation

Org Lett. 2013 Apr 5;15(7):1776-9. doi: 10.1021/ol400639m. Epub 2013 Mar 22.

Abstract

The homogeneous catalyzed dehydrogenation of methanol in a synthetically valuable cross-coupling reaction was achieved. By the use of a simple ruthenium-N-heterocyclic carbene complex, MeOH and primary or secondary amines can be converted into formamides.