Nonresonant background suppression in coherent anti-Stokes Raman spectroscopy through cascaded nonlinear optical interactions

Opt Lett. 2013 May 1;38(9):1551-3. doi: 10.1364/OL.38.001551.

Abstract

We propose and experimentally validate a technique for four-wave mixing background suppression in coherent anti-Stokes Raman spectroscopy. It is based on the interaction of the signals generated from the Kerr third-order nonlinearity and the cascaded quadratic process in a nonlinear crystal. Theoretical analysis agrees well with the experimental results, which provide a quantitative assessment of different contributions and allow extraction of the nonlinearity parameters.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Nonlinear Dynamics*
  • Optical Phenomena*
  • Spectrum Analysis, Raman / methods*