Self-sufficient and exclusive oxygenation of methane and its source materials with oxygen to methanol via metgas using oxidative bi-reforming

J Am Chem Soc. 2013 Jul 10;135(27):10030-1. doi: 10.1021/ja405439c. Epub 2013 Jul 1.

Abstract

A combination of complete methane combustion with oxygen of the air coupled with bi-reforming leads to the production of metgas (H2/CO in 2:1 mole ratio) for exclusive methanol synthesis. The newly developed oxidative bi-reforming allows direct oxygenation of methane to methanol in an overall economic and energetically efficient process, leaving very little, if any, carbon footprint or byproducts.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Carbon Monoxide / chemical synthesis
  • Carbon Monoxide / chemistry*
  • Hydrogen / chemistry*
  • Methane / chemistry*
  • Methanol / chemical synthesis*
  • Methanol / chemistry
  • Oxidation-Reduction
  • Oxygen / chemistry*

Substances

  • Carbon Monoxide
  • Hydrogen
  • Methane
  • Oxygen
  • Methanol